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Realtime correction of probe pulse in subpicosecond time-resolved transient absorption spectroscopy
ZhangSu-Juan; DuanCun-Li; FengXiao-Qiang; HeJun-Fang; Zhang Sujuan
2011
会议名称International Symposium on Photoelectronic Detection and Imaging 2011: Laser Sensing and Imaging; and Biological and Medical Applications of Photonics Sensing and Imaging
会议录名称Proceedings of SPIE - The International Society for Optical Engineering
页码81923P
会议日期May 24, 2011 - May 26, 2016
会议地点Beijing, China
出版地P.O. Box 10, Bellingham, WA 98227-0020, United States
出版者SPIE
会议主办者Chinese Society of Astronautics (CAS)
产权排序3
摘要Due to its breakthrough the electro-optical time response limitation for picosecond dynamics of processes, many research groups around the world operating in different fields from physics and chemistry to biology, medicine and material science, utilize laser setups capable of providing subpicosecond pulses and femtosecond-level time delay lines. However the signal amount of Femto-picosecond Dynamics is about at an altitude of 1%, but the fluctuation of femtosecond probe pulse at its best can only reach about 5%. Real-time correct the probe pulse is the only effective way to realize subpicosecond time-resolved detection precision of transient absorption spectroscopy. So in this paper, reference pulse was drawn into the measurement equipment through different methods to dispel the fluctuation of probe pulse. Firstly, in the case of Subpicosecond time-resolved transient absorption spectroscopy, probe and reference beams have the same spectral distribution and derived from the same source to measure the variation of transmittance in the excited volume. Secondly probe pulse is spatially and temporally overlapped to the excitation pulse, reference pulse spatially overlapped but temporally anticipated in respect to the excitation pulse. Finally reference pulse passes through the sample in a different position. The detector can be a CCD camera or a double photodiode. The results shown that when reference pulse passes through the sample in a different position and detected by CCD, the correction results can reach to 1%. Which meet the femto-picosecond dynamics precise requirement.
关键词Realtime Correction Probe Pulse Reference Pulse Subpicosecond Time-resolved Transient Absorption Spectroscopy
作者部门瞬态光学国家重点实验室
收录类别EI
语种英语
ISSN号0277-786X
文献类型会议论文
条目标识符http://ir.opt.ac.cn/handle/181661/20192
专题瞬态光学研究室
通讯作者Zhang Sujuan
推荐引用方式
GB/T 7714
ZhangSu-Juan,DuanCun-Li,FengXiao-Qiang,et al. Realtime correction of probe pulse in subpicosecond time-resolved transient absorption spectroscopy[C]. P.O. Box 10, Bellingham, WA 98227-0020, United States:SPIE,2011:81923P.
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