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Mechanism of All-Optical Spatial Light Modulation in Graphene Dispersion
Liu, S1,2; Han, J1; Cheng, XM1,2; Wang, X2; Zhang, Q3; He, B1; Jiao, TF1; Ren, ZY1
作者部门瞬态光学研究室
2021-08-05
发表期刊JOURNAL OF PHYSICAL CHEMISTRY C
ISSN1932-7447;1932-7455
卷号125期号:30页码:16598-16604
产权排序1
摘要

Graphene is a superb material with significant potential in broadband all-optical modulation. However, the mechanism of the all-optical modulation in graphene dispersion is still under debate. Here, we report on a pump power-dependent spatial light modulation by using the 780 nm CW laser as the pump and signal beams via graphene dispersion. The results indicate that graphene is able to convert the Gaussian signal beam into a hollow beam with a ring pattern. Examining the temporal evolution of the ring pattern, we found that spatial cross-phase modulation (SXPM) plays the dominant role at low pump power, while nonlinear scattering (NLS) becomes dominant when the pump power is high. Furthermore, the dependence of the size and intensity of the signal ring pattern on the pump power is investigated. The results can be well explained by SXPM, NLS, and saturation absorption (SA) effects. Finally, an all-optical switch is developed based on the dependence of the signal intensity on the pump power. It is demonstrated that both in-phase and out-phase modulation can be realized in one system. This work not only provides useful information in understanding the mechanism of graphene in interacting with the light, but also suggests a new way to produce hollow beam with tunable size and achieve an all-optical switch with both inphase and out-phase modulation.

DOI10.1021/acs.jpcc.1c04423
收录类别SCI ; EI
语种英语
WOS记录号WOS:000683810700027
出版者AMER CHEMICAL SOC
EI入藏号20213310767949
引用统计
被引频次:4[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.opt.ac.cn/handle/181661/94999
专题瞬态光学研究室
通讯作者Cheng, XM
作者单位1.Northwest Univ, Int Collaborat Ctr Photoelect Technol & Nano Func, Inst Photon & Photon Technol, State Key Lab Photon Technol Western China Energy, Xian 710069, Peoples R China
2.Chinese Acad Sci, State Key Lab Transient Opt & Photon, Xian 710119, Peoples R China
3.XIAN Univ Posts & Telecommun, Sch Elect Engn, Xian 710121, Peoples R China
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Liu, S,Han, J,Cheng, XM,et al. Mechanism of All-Optical Spatial Light Modulation in Graphene Dispersion[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2021,125(30):16598-16604.
APA Liu, S.,Han, J.,Cheng, XM.,Wang, X.,Zhang, Q.,...&Ren, ZY.(2021).Mechanism of All-Optical Spatial Light Modulation in Graphene Dispersion.JOURNAL OF PHYSICAL CHEMISTRY C,125(30),16598-16604.
MLA Liu, S,et al."Mechanism of All-Optical Spatial Light Modulation in Graphene Dispersion".JOURNAL OF PHYSICAL CHEMISTRY C 125.30(2021):16598-16604.
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