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Coherence in ultrafast laser-induced periodic surface structures
Zhang, Hao1; Colombier, Jean-Philippe1; Li, Chen1,2,3; Faure, Nicolas1; Cheng, Guanghua2; Stoian, Razvan1; Zhang, H
作者部门瞬态光学技术国家重点实验室
2015-11-13
发表期刊PHYSICAL REVIEW B
ISSN1098-0121
卷号92期号:17页码:174109
产权排序2
摘要Ultrafast laser irradiation can trigger anisotropically structured nanoscaled gratinglike arrangements of matter, the laser-induced periodic surface structures (LIPSSs). We demonstrate here that the formation of LIPSS is intrinsically related to the coherence of the laser field. Employing several test materials that allow large optical excursions, we observe the effect of randomizing spatial phase in generating finite domains of ripples. Using three-dimensional finite-difference time-domain methods, we evaluate energy deposition patterns below a material's rough surface and show that modulated pattern, i.e., a spatially ordered electromagnetic solution, results from the coherent superposition of waves. By separating the field scattered from a surface rough topography from the total field, the inhomogeneous energy absorption problem is reduced to a simple interference equation. We further distinguish the contribution of the scattered near field and scattered far field on various types of inhomogeneous energy absorption features. It is found that the inhomogeneous energy absorption which could trigger the low-spatial-frequency LIPSSs (LSFLs) and high-spatial-frequency LIPSSs (HSFLs) of periodicity Lambda > lambda/Re((n) over tilde) are due to coherent superposition between the scattered far field (propagation) and the refracted field, while HSFLs of Lambda > lambda/Re((n) over tilde) are triggered by coherent superposition between the scattered near field (evanescent) and the refracted field. This is a general scenario that involves a topography-induced scattering phenomenon and stationary evanescent fields, being applied to two model case materials that exhibit large optical excursions upon excitation (W, Si) and nonplasmonic to plasmonic transitions. We indicate the occurrence of a general light interference phenomenon that does not necessarily involve wavelike surface plasmonic excitation. Finally, we discuss the role of interference field and scattered field on the enhancement of LIPSSs by simulating interpulse feedback effects and provide the electromagnetic origin of grooves (Lambda > lambda) related to a feedback-driven topography evolution. Those results strongly suggest the electromagnetic interpretation of LIPSSs in interplay with an evolving surface topography.
文章类型Article
学科领域Physics, Condensed Matter
WOS标题词Science & Technology ; Physical Sciences
DOI10.1103/PhysRevB.92.174109
收录类别SCI
关键词[WOS]FEMTOSECOND LASER ; PULSES ; ABLATION ; RIPPLES ; MORPHOLOGY ; SILICON
语种英语
WOS研究方向Physics
项目资助者French National Research Agency (ANR) project DYLIPSS(ANR-12-IS04-0002-01) ; China Scholarship Council
WOS类目Physics, Condensed Matter
WOS记录号WOS:000368094200001
引用统计
被引频次:73[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.opt.ac.cn/handle/181661/27793
专题瞬态光学研究室
通讯作者Zhang, H
作者单位1.Univ St Etienne, Univ Lyon, UMR CNRS 5516, Lab Hubert Curien, F-42000 St Etienne, France
2.Chinese Acad Sci, Xian Inst Opt & Precis Mech, State Key Lab Transient Opt & Photon, Xian 710119, Shaanxi, Peoples R China
3.Univ Chinese Acad Sci, Beijing 10049, Peoples R China
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GB/T 7714
Zhang, Hao,Colombier, Jean-Philippe,Li, Chen,et al. Coherence in ultrafast laser-induced periodic surface structures[J]. PHYSICAL REVIEW B,2015,92(17):174109.
APA Zhang, Hao.,Colombier, Jean-Philippe.,Li, Chen.,Faure, Nicolas.,Cheng, Guanghua.,...&Zhang, H.(2015).Coherence in ultrafast laser-induced periodic surface structures.PHYSICAL REVIEW B,92(17),174109.
MLA Zhang, Hao,et al."Coherence in ultrafast laser-induced periodic surface structures".PHYSICAL REVIEW B 92.17(2015):174109.
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