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Magnetic properties and photoluminescence of thulium-doped calcium aluminosilicate glasses
So, Byoungjin1; She, Jiangbo1,2,3; Ding, Yicong1; Miyake, Jinsuke4; Atsumi, Taisuke4; Tanaka, Katsuhisa4; Wondraczek, Lothar1,5
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2019-11-01
发表期刊OPTICAL MATERIALS EXPRESS
ISSN2159-3930
卷号9期号:11页码:4348-4359
产权排序3
摘要

We report on the optical and magnetic properties of Tm2O3-doped calcium aluminosilicate glasses with dopant concentrations of up to 7 mol%. These materials provide a rare case in which high magnetic susceptibility, low Faraday rotation, Tm3+-related infrared photoluminescence and the ability to produce optical fibers are combined. From emission intensity and decay curves of the H-3(4)-> F-3(4) and (3)F4 -> H-3(6) transitions, we find cross-relaxation already for 0.5 mol% of Tm2O3 doping, indicating notable Tm2O3 clustering. This facilitates antiferromagnetic interaction and results in high magnetic susceptibility. Substitution of Al2O3 by Tm2O3 induces a more asymmetric local structural environment around Tm3+ species and enhances the diamagnetic contribution to Faraday rotation as opposed to the other rare-earth ions. (C) 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

DOI10.1364/OME.9.004348
收录类别SCI ; EI
语种英语
WOS记录号WOS:000493994700021
出版者OPTICAL SOC AMER
EI入藏号20195107878498
引用统计
被引频次:9[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.opt.ac.cn/handle/181661/31911
专题信息中心
通讯作者Wondraczek, Lothar
作者单位1.Friedrich Schiller Univ, Otto Schott Inst Mat Res, Fraunhoferstr 6, D-07743 Jena, Germany
2.Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Xian Inst Opt & Precis Mech, State Key Lab Transient Opt & Photon, Xian 710119, Shaanxi, Peoples R China
4.Kyoto Univ, Grad Sch Engn, Dept Mat Chem, Kyoto 6158510, Japan
5.Univ Jena, Abbe Ctr Photon, Albert Einstein Str 6, D-07743 Jena, Germany
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So, Byoungjin,She, Jiangbo,Ding, Yicong,et al. Magnetic properties and photoluminescence of thulium-doped calcium aluminosilicate glasses[J]. OPTICAL MATERIALS EXPRESS,2019,9(11):4348-4359.
APA So, Byoungjin.,She, Jiangbo.,Ding, Yicong.,Miyake, Jinsuke.,Atsumi, Taisuke.,...&Wondraczek, Lothar.(2019).Magnetic properties and photoluminescence of thulium-doped calcium aluminosilicate glasses.OPTICAL MATERIALS EXPRESS,9(11),4348-4359.
MLA So, Byoungjin,et al."Magnetic properties and photoluminescence of thulium-doped calcium aluminosilicate glasses".OPTICAL MATERIALS EXPRESS 9.11(2019):4348-4359.
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